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You can buy "Curious George 3: Back to the Jungle" on Apple TV as download or rent it on Apple TV online.
When Curious George is offered a special space mission, Ted (The Man in the Yellow Hat) can't deny his little friend this exciting journey, especially after Curious George completes the training. But when he crash-lands in Africa, a worried Ted goes searching, expecting the worst, only to have it turn out to be the best.