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Currently you are able to watch "Lupin the Third: The Secret of Twilight Gemini" streaming on Tubi TV for free with ads or buy it as download on Amazon Video. It is also possible to rent "Lupin the Third: The Secret of Twilight Gemini" on Amazon Video online
As Lupin's mentor Don Dolune lies on his deathbed, he hands the master thief a gift, the diamond named Twilight. Though it's only half the treasure — the other half of the Twilight can be found in Morocco. Lupin must contend with his on-again-off-again-partner Fujiko, his feelings for the mysterious Lara, and the relentless whip-wielding maniac Sadachiyo in order to bring Twilight back to its full glory.