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You are able to buy "The Girl from U.N.C.L.E." on Apple TV, Amazon Video, Google Play Movies as download.
The Girl from U.N.C.L.E. is an American spy-fi TV series that aired on NBC for one season from September 16, 1966 to April 11, 1967. The series was a spin-off from The Man from U.N.C.L.E. and used the same theme music composed by Jerry Goldsmith, which was rearranged into a slightly different, harder-edged arrangement by Dave Grusin.